First go to COLLECTIONS, and select the one you want to delete the book from (in your case "Unread"). Then hit the OPTIONS button, and one of the choices will be Remove Content. Tap that and all of the books in the collection appear with little boxes by them; tap the one(s) you want to delete (a check mark will appear in the box), then hit DONE in the upper right corner. The last step is essential - kind of like hitting SAVE to save your work.
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