I've had the same problem — sometimes sync would work fine, and other times it would hang forever and I'd have to exit the Reader Library program. So I cleared all the sync checkboxes and don't depend on it at all, just drag new books onto the "Reader" line in Reader Library. When I'm ready to delete a book (such as an expired public library book), they can be deleted from the Reader either through the Reader Library program or directly from the Reader after it's disconnected. This means I don't transfer any "collections" onto the Reader, but I don't find that's a major loss. Most of what I read is from the public library anyway.
Ned
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