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Sync - It might be, but you only see the sync options when the reader is connected, so be sure to check then.
(Relatively) small numbers of books on seperate cards is probably the best way to go if you need then available without a PC. Personally, I just tend to have a small number of books on the Reader (100 or so), but use Calibre to manage the library/reader.
Was there any particular issue with Calibre?
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