You may also want to move your calibre library outside your Documents folder since Microsoft has been doing security changes in the default permissions on Documents and with their synchronizing to One Drive.
Close calibre, move the library folder in C:\Users\<username>, re-open calibre and under Library dropdown menu, select the Switch/create library, browse to your new library location and make sure that the radio button for Use the previously existing library at the new location is selected.
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