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Only if you keep your library in a cloud storage (I keep mine in Dropbox). But since a Calibre library is not really meant to be accessed from several different computers, it's easily corrupted. You must always pause the background syncing when you open Calibre, and you can only have one instance of your library open at once, anywhere. Also you should run the library check often, because mistakes do happen. If you ignore these rules, you'll end up with a messed up library very quickly. So most people don't use their library this way.
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