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One thing to think about is moving your Calibre library folder from Documents to the root of your User folder. There have been several issues with having the Calibre library in the Documents folder when Windows Defender's Controlled Folder Access detects Calibre's actions as a ransomware attack.
I'd suggest closing Calibre, moving the Calibre library folder from \Users\<User name>\Documents\Calibre to \Users\<User name>\Calibre. Open Calibre and use the Switch/Create Library to connect to the library at it's new location (make sure you select Use the previously existing library at the new location button).
Once that is done and you are happy with the new location, select the library in the root of your C: drive, select all books and copy to your main calibre library. This may result in message about duplicate books. I'd suggest not copying the duplicates but rather manually checking and deciding which duplicate you want to keep if they are duplicates.
Once you have the libraries consolidated, you can remove the library from the root of your C: drive.
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