I replied to your post in another thread, but, I'll add it here as well.
To the best of my knowledge, the answer no. The Goodreads Sync plugin can sync shelves and reading progress between calibre and Goodreads. It can also set a review. It doesn't do quotes. From memory, the request has been made before and I had a look at it. And if I remember correctly, the GR API doesn't have this as a function. Even with an API, it would be a reasonable amount of work to implement. It is also not something that I am personally interested in. As such, it isn't something I have an interest in implementing, but, if someone was, I would be happy to help.
Note: I am not the original author of the Goodreads Sync plugin. But, I have been maintaining it as necessary for the last few years.
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