For pBooks, I've scanned them all into LibraryThing.
Very useful if you are browsing secondhand bookshops, as you can search online to check what you do and don't already have.
Was a godsend when moving house, as I could tag each book with what box it was stored in.
I started off doing that for eBooks too, but don't really feel the need now. I can just carry my entire library on my phone, so don't need access to just a list of books.
For eBooks I import them all into Calibre, make sure the author and titles are in the 'correct' (for me) formats, and that everything is organised by genre and series, then run them through a process that converts each series to a single book for transfer to my readers. I find it easier to browse things on a small-screen device that way.
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