Once upon a time, Calibre Portable did not exist so people created and used the batch file to make normal Calibre portable. You can use the batch file with Calibre Portable's directory structure, though, with some minor modifications (need to fix the paths).
The folder "\Calibre Portable\Calibre" already contains the normal 32-bit Windows Calibre install. It's calibre-portable.exe that handles all the portabilization.
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