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Not everyone will agree, but I find that these catalog-management applications, like Calibre for books or MediaMonkey for music, make much more sense if you use the full application on a PC or Mac, where having a bigger screen makes the app more productive, and a companion smartphone app, like Calibre Companion, to browse the library from a smartphone.
There is also the question of where to store the data (books) you are organising.
I wouldn't want to store it on a phone. I could keep the data on Dropbox or on a NAS and connect the phone, but why? I see many downsides in running Calibre from a phone vs a PC, but not many advantages.
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