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No, Calibre is a Windows/Mac/Linux program for Desktop/Laptop computers. The are apps like Calibre Companion which can connect to Calibre wirelessly or to the Calibre server and transfer books to the tablet, but not full on Calibre. CC does have similar tag browsing & sorting to Calibre though so can be a nice "library" app (it works in conjunction with a users preferred reading app, but does not contain a reading app of its own).
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