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That's an error sending a file to the device. You can try rebooting botht he device and your computer, that sometimes fixes this kind of error. If not,
1) You can try a different usb cable/port
2) You can try resetting your device (though this will wipe everything from it)
3) You can use one of th ewireless transfer methods described in the calibre FAQ
You cannot choose which folders on the device to scan until calibre has connected the first time to the device.
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