@HeatherMC - to remove a book from the library hit the delete key in calibre. To remove a file from the My Documents folder, hit the delete key in Windows/File explorer (shift/del to delete permanently). In both cases you can select multiple items.
Calibre doesn't have a permanent delete capability - ie no shift/del - its always deletes to the Recycle bin. When calibre does book deletions it moves the data to transient folders which are then sent to the Recycle bin. So to get that space back you must either delete those folders from the Recycle bin, or empty the Recycle bin entirely.
BR
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