Tell CC the name of the folder where your book are (in the "Formats and folders" setting), and make sure the "Scan on connect" option is checked in CC's settings. When you wirelessly connect to Calibre it will then scan the folder to find what books you have, and retrieve the metadata for them wirelessly from Calibre. After it's finished the initial data retrieval (which will take a while for a large library), go into Settings again and uncheck the "Scan on connect" box.
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