Well, there are a few options I can think of...
Put the library in "the cloud" using a service like DropBox, Box or Copy and point Calibre to it (this would make a local copy of the books on each machine, also would give you some backups in case something happened to one of the machines).
Share your Desktop drive and map the drive from her laptop and point Calibre to the library on it. Or setup some other network hard drive and connect both Calibre installs to that.
With either option make sure only one of you is accessing it at a time.
Setup Calibre Content Server and have her access books that way.
Or just copy the library over to her computer each time you make a change. Make sure changes are only made from one machine.
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