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calibre.exe is using 800MB a 32 bit process on windows can allocate a max of 2GB if it is running out of memory that implies it is trying to allocate a further 1.2GB, I dont see how that's possible while writing metadata.calibre, since all that file contains is a cache of metadata. How many books in your library, how many are you sending to the device?
Try creating a new empty library add one or two books and send those to the folder and see what happens.
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