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Not as I know of. At least not if your device itself doesn't allow it.
Note that allowing this sort of thing would, in my (admittedly personal) view, be a Bad Thing: how would you know which metadata version would hold true? Especially after a few weeks (or even days), and you've forgotten even why you made the changes. Better to do all the work in Calibre, then update your device if necessary. This is, after all, what Calibre is for.
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