I put it there because that's where I thought I'd been told was the best place for it (in the "I thought Portable meant Portable - It Doesn't " thread,) but when I went and checked I realised I must have read it wrong.
I've deleted all the files of the previous portable version downloaded the full x64 version and installed to the default location, it installs fine but when I try and open the program I get the same error message as above... So now I have the full version looking in the location of the old portable version!
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