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Not possible, sorry.
You use calibre to prepare and convert and then send books to the device. And then a reading app on the device to read the books.
You can access a computer running calibre from the device, using a remote desktop program or the calibre server via a webbrowser or a reading app with opds support, for instance Mantano Reader.
I send my books from my computer to a shared folder on a NAS. And copy the books from there over wifi using my Xoom tablet and the app FolderSync.
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