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Connect your iPhone to your computer, and open iTunes>Info Tab.
If contacts and calendar are set to iCloud, you will see "Your contacts are being synched with your iPhone over the iCloud. Over the air settings can be changed on your iPhone."
On the iPhone, go to Settings>iCloud, and you may find that your Contacts and Calendars are set to sync with iCloud (the setting is "ON"). If you turn one or more of these settings "OFF", you will be asked whether you want to delete the data on the iPhone. You can choose whether you want this, but for me, I kept the data on the iPhone that had previously been synced with iCloud.
You'll notice that upon taking this step, you now have the option to sync your Contacts and Calendar to Outlook.
Good luck!
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