I'd dump all of them into a folder somewhere on your hard drive, and remove them from Calibre. If you're looking for something new to read, then look in that pile first, and if you find something you like, import it into Calibre. I do it this way: every book I've got in Calibre has been read, or will certainly be read. All the rest is stored somewhere else, which is basically a huge bunch of classics of which I don't know if I will ever read (all of) them.
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