What I did was copy the whole library folder and put it on the new hardrive where I wanted it (I use dropbox, so I just waited for my dropbox folder to sync, which took leaving it overnight). Then I downloaded Calibre. When I started it, there was an option to create a new library using a folder you have already (as opposed to having Calibre create one). I chose that and within a minute or two, all my books were there as I had left them. Very easy!
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