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I think this is right, someone will correct me if it's not.
Copy your Calibre Library to your Dropbox folder, then open Calibre and select the Library button at the top (looks like the Calibre icon).
Select 'Switch/Create Library' and navigate to the Dropbox folder, select your library, hit Ok, and Dropbox will automatically sync any changes you make with your online backup.
You can delete your old library once you're sure it's all working.
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