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By catalogs I'm going to assume you mean your actual library or do you mean the catalogs generated from the Convert Books button?
If it's the second one, Convert Books generated catalogs, then all you need to do is tell Calibre to save them in your Dropbox when you create them.
If you mean your actual library then NO, do NOT do any of the steps you just listed. What you actually want to do is click on the Books icon as shown in the first attached picture and then select Switch/Create Library. Then, as you see in the second attached picture, you tell Calibre the new location in your Dropbox where you want your library stored, select Move Current Library To New Location and then click OK. This will safely move your library to its' new home.
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