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No you cannot re-sort by title in that dialog. The changing of list order with the buttons would not work if I allowed that.
If you want to view by title, then just choose the View List option in the menu. This will put the books in your library view. Initially they will be sorted by the same order as the edit dialog (i.e. your list sequence) but you can click on the title column to see them in a different order.
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