If you are using SugarSync in local mode then you should be able to find the SugarSync folder under My Documents (assuming you are using Windows). From there you should be able to do any normal file related operations. If you are using Shared folders then if you are not the owner this does not seem to work - you have to operated via the SugaSync File Manager.
A requirement for Calibre2opds ''over the-air' access (which since you mention the iPad I think is what you really want to do?) is that the syncing software must expose a 'base URL' that is the Calibre Library, and that it must be possible to reference all book files and catalog files as being relative to this URL. In Dropbox this can be done via the users Public folder. I am not certain that SugarSync provides an equivalent facility?
I might have a more detailed look at SugarSync myself to see if I can see how it might be used with Calibre2Opds as I have both installed in my test environment. In my live environment I have been using DropBox as it seemed much less fiddly to manage, and consumed far less resources on my PC. Also Dropbox allowed my to put the MyDropbox folder on any drive while SugarSync seemed to insist that the Magic briefaces was located under My Documents. However thiese observations could simply due to my lack of knowledge on how SugarSync works.
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