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You should be able to transfer books over with the SONY Reader Library. I do it all the time, both ways (purchase stuff on the device and transfer it to my pc and other way around).
Not sure what kind of problem you are having.
One possibility is that the Reader Library is not registered/authenticated or whatever they call that... and hence you can't transfer to it. Open the software, go to the store, open your account ('manage my account' or whatever) then click on "Manage/Rename Devices" under "My devices". You should see your PC there. If not, follow the on-screen instructions to add it. You can only have 1 PC and 2 devices authorized at the same time on the same account.
Another possibility is that you are not dragging to the right spot when 'dragging and dropping'. IF you try to drop a book from a device into a collection in your Library, it won't work. You have to drag and drop it into the actually "Library". Then, from there, you can transfer it to a collection.
I had problems with synch as well. It works when I transfer content from the PC to the device, but it sometimes won't work the other way around, even if I select the correct options from the settings.
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