If you look on your Kindle you should see 'Archived Items' on the home page. Go into this and you will see your books that were bought before your got your K3. At least, that's where mine are. You can select the proper book and it will download it.
Or you can go into your Amazon account and go to 'manage your Kindle' and just push all your books from there.
Since you have the book for Apple4Mac already there is no need to involve Calibre, unless you want to. And the book should still be on your computer, also, either way.
If you already started reading your might need to sync, but I am unsure, since I just got my K3, as well.
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