Calibre supports Android devices; however, its support is probably rudimentary. Your best bet is transferring the files like in any USB stick, and using apps like Aldiko, FBReaderJ or CoolReader to read them. In spite of the slight inadequacy of SlowRain's posts, his point is valid: cloud storage solutions like DropBox or SpiderOak have the advantage that you can keep your folder structure exactly as you want to: that is, you can take your Calibre Library and copy it into your Dropbox desktop folder provided that it takes less than 2 gigabytes or that you pay the Dropbox fees; nevertheless, the Dropbox Android app won't download the whole library on your phone, but it'll download the files in an on-request basis.
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