A single reason to use the Sony Reader software - Dragging books into Collections.
I use Calibre for my free ebooks and ADE for my store-bought ones, but unfortunately Calibre can't add tags (which become Collections in the 600) to some DRM books. Fortunately you can use the Sony Reader software to drag even DRM'ed books into Collections. This can also be useful if you need to move a lot of books into a Collection; you can Shift select and drag them all at once.
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