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Never quite thought of it like that, but, Kindle for PC and Nook for PC are the applications recommended for managing books/collections for their devices via PC, and in the case for Kindle, especially for transferring library books. Many of the books in Overdrive cannot be synced wirelessly, but must be transferred via PC.
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Transferring Kindle library books "via PC" doesn't involve Kindle for PC at all. "Transferring via PC" means precisely that... you manually download the file to your PC and transfer it to your Kindle like you would copy/move a file to any USB device. In fact, Kindle for PC/Mac has nothing to do with a Kindle device ever, really (other than sharing some meta-stuff like archive/collections, bookmarks/highlights, and furthest read point). Kindle for X, is really only used for
reading your ebooks on X. Definitely not for transferring ebooks to other devices.