I know it's not the popular choice with MR members, but I much prefer LibraryThing over GoodReads. I wouldn't necessarily suggest that anyone who has an established GR presence switch over to LT, but if (like OP) you haven't really gotten started I most definitely advice you to check out LibraryThing before making your choice.
I was aware of both options when I decided I wanted some kind of online mechanism for keeping track of my books and finding new things to read. I signed up for GoodReads first because I preferred the visual design of that site to LibraryThing's. After having used GoodReads for a while, I discovered I didn't like the general mechanics of the site, as well as the inability/difficulty to edit book profiles to suit my preference.
I then checked out LibraryThing and it was much more up my alley, and so I never went back to GoodReads.
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